RCQM/FCMP: Yu-Ping Lin: Rich electronic phase diagram in kagome flat band
TLDRThe speaker from UC Berkeley presents a detailed exploration of electronic phases in frustrated Kagome lattice materials, focusing on the effects of repulsive electrons on flatbands. Through mean-field analysis, various novel magnetic and charge orders are discovered, including stripe orders and non-colinear spin structures. The talk suggests that by reducing on-site repulsion in materials like iron germanium, it may be possible to observe non-collinear magnetic orders. The speaker also proposes that beyond mean-field theory, there could be potential for quantum spin liquids and unconventional superconductivity, with ongoing research to explore these possibilities.
Takeaways
- ๐ The speaker, Dring Lin from UC Berkeley, is presenting on the topic of electronic phases in kagome lattice materials, particularly focusing on the effects of repulsive electrons on flatbands.
- ๐งฒ Dring Lin's work is based on a mean-field theory analysis of the kagome flatband, revealing various interesting electronic phases that arise under different conditions of electron repulsion.
- ๐ฌ The presentation includes a detailed analysis of the flatband across different fillings, showing a progression from ferromagnetism to various stripe and non-collinear spin orders as the filling changes.
- ๐ The speaker acknowledges the contribution of their advisor and colleagues, emphasizing the collaborative nature of the research and the use of mean-field theory for the analysis.
- ๐ญ The research explores the possibility of observing different electronic phases in experiments, with a focus on locating iron and iron germanium within the phase diagram to understand observed behaviors.
- ๐งฌ The mean-field theory analysis was extended to include on-site and nearest-neighbor repulsion, revealing additional phases such as quantum spin Hall insulators and charge density waves.
- ๐ The potential relevance to real-world materials is discussed, with suggestions that reducing the Coulomb repulsion in materials could lead to the observation of non-collinear spin orders or stripe orders.
- ๐ The speaker also speculates on what could happen beyond mean-field theory, suggesting the possibility of observing Z2 spin liquids and other exotic states with further research.
- ๐ The presentation includes a comparison of the theoretical findings with experimental results, particularly focusing on iron and iron germanium materials and their magnetic properties.
- ๐ The speaker concludes by summarizing the findings and suggesting future research directions, including the use of beyond mean-field techniques to explore the potential for fractional excitations and unconventional superconductivity.
Q & A
What is the main topic of Dr. Lin's talk from UC Berkeley?
-Dr. Lin's talk is focused on the story of Kagome lattice flatbands and the discovery of interesting electronic phases within this context.
What is the significance of flatbands in condensed matter physics?
-Flatbands are significant because they can host very strong interacting electron phases, and they are usually accompanied by high tunability in terms of doping or band structure, which can lead to various experimentally observable phenomena.
What are the two ways to enhance the interaction electron base in a flatband system?
-The two ways to enhance the interaction electron base in a flatband system are to increase the interaction U, which expands the interacting window, and to narrow the bandwidth, which involves more electronic states given a fixed interacting window.
What is the role of frustration in Kagome lattice systems?
-In Kagome lattice systems, frustration leads to the formation of compact localized states, which are the elements of the flatbands. These states arise due to destructive interference of hopping, which can result in zero density after hopping.
What are some examples of frustrated materials that exhibit flatbands?
-Examples of frustrated materials that exhibit flatbands include kagome lattices like herbertsmithite (ZnCu3(OH)6Cl2), paracanthite (PbCu3(OH)6Cl2), and linarite (PbCu3(OH)6SO4).
What is the relevance of the mean-field theory in understanding interacting electrons on a flatband?
-Mean-field theory is used to simplify the complex problem of interacting electrons on a flatband by mapping it onto an effective single-particle Hamiltonian. This approach allows for the analysis of the ground state and the identification of possible symmetry-breaking orders.
How does the introduction of extended repulsion in the model affect the electronic phases?
-The introduction of extended repulsion can lead to additional electronic phases such as quantum spin Hall insulators, charge density waves, and various types of antiferromagnetic and non-collinear spin orders.
What is the significance of the half-filled flatband in the context of Dr. Lin's research?
-The half-filled flatband is significant because it is a regime where ferromagnetism is expected to occur, and it is a point of interest for studying the stability of different magnetic orders and the potential for other electronic phases.
How does the Kagome flatband model differ when considering only on-site repulsion versus including extended repulsion?
-When considering only on-site repulsion, the model focuses on nearest-neighbor hopping and on-site interaction, leading to specific magnetic orders. Including extended repulsion introduces additional complexity and can result in a variety of new phases, including non-collinear spin orders and charge density waves.
What experimental relevance does Dr. Lin's work have for materials like iron germanium?
-Dr. Lin's work suggests that by tuning the interaction parameters in materials like iron germanium, it may be possible to observe non-collinear spin orders or stripe orders that are predicted by the mean-field analysis of the Kagome flatband model.
Outlines
๐ Introduction and Background
The speaker introduces Dr. Lin from UC Berkeley, who is giving a talk on his postdoctoral research. Dr. Lin obtained his PhD from the University of Colorado and is now working at UC Berkeley. The talk focuses on the discovery of unique electronic phases in kagome lattice materials, particularly focusing on the repulsive electrons on the flatband. The speaker also acknowledges the support from the Birley group and the CMT group at the University of Bristol, where the work was conducted under the supervision of advisor Joe Mo.
๐ฌ Electron Interactions and Symmetry Breaking
This paragraph delves into the behavior of interacting electrons in a crystal lattice. It explains how electrons form bands due to dispersion energy and how interactions can lead to symmetry breaking and the emergence of different ground states. The speaker discusses the concept of an order parameter and how it can be used to characterize symmetry breaking in systems such as ferromagnetism, charge density waves, and superconductivity. The strength of the interaction phase is estimated by the number of electronic states within the interaction window, which is defined by the interaction strength and the band width.
๐ Flatbands and Frustrated Lattices
The speaker explores the concept of flatbands and their significance in frustrated lattice systems. Flatbands occur when the bandwidth vanishes, leading to a very strong interaction electron phase. The interest in flatbands has grown due to their potential to host strongly correlated electron phases and their high tunability through doping or magnetic fields. The speaker highlights the kagome lattice as a prime example of a frustrated system that can host flatbands due to destructive interference in electron hopping.
๐ Kagome Materials and Electron Phases
This section focuses on kagome materials and their properties, particularly the presence of flatbands close to the Fermi level. The speaker discusses the binary materials TX, where T could be iron, molybdenum, or cobalt, and X could be germanium or silicon. These materials exhibit intralayer ferromagnetism and charge density waves. The speaker also mentions the tunability of the Fermi level in these materials through elemental substitution, which can lead to the observation of various electron phases in experiments.
๐ฌ Mean-Field Theory and Electron Repulsion
The speaker introduces the mean-field theory (MFT) as a method to analyze the behavior of repulsive electrons on the flatband. The Hartree-Fock approximation is used to map the interacting electron problem onto an effective single-particle problem. The speaker discusses the limitations of previous MFT analyses and presents a more comprehensive approach that does not impose constraints on the wave function, allowing for a more accurate determination of the ground state and symmetry breaking orders.
๐ Discovery of New Magnetic Orders
In this paragraph, the speaker presents the results of their comprehensive Hartree-Fock analysis, which reveals a variety of new magnetic orders across the flatband. These include stripe and non-collinear spin orders that have not been previously reported in the literature. The speaker also discusses the importance of the 120-degree spin order in the face diagram and how their analysis differs from previous studies.
๐ Phase Diagram and Material Relevance
The speaker discusses the phase diagram resulting from their analysis and attempts to relate their theoretical findings to practical materials like iron and iron germanium. They propose that by reducing the Coulomb repulsion in these materials, it might be possible to observe non-collinear and stripe orders. The speaker also suggests that current materials may be in a strongly repulsive regime, which could be why certain orders are not observed experimentally.
๐ฎ Beyond Mean-Field Theory
In the final part of the talk, the speaker speculates on what could be observed beyond the mean-field level, such as quantum spin liquids, fractional excitations, and unconventional superconductivity. They mention ongoing work using techniques like the density matrix renormalization group (DMRG) to explore these possibilities and express hope for future discoveries.
๐ค Questions and Discussion
The final paragraph consists of a Q&A session where the audience asks questions about the ordering vectors of different phases, the topological aspects of the bands, and the experimental relevance of the findings. The speaker addresses these questions, providing insights into the stability of the states, the potential impact of considering band topology, and the expected changes in the band structure for different materials.
Mindmap
Keywords
๐กPostar
๐กUC Berkeley
๐กFlatband
๐กInteraction electrons
๐กSymmetry breaking
๐กFrustrated systems
๐กCompact localized states
๐กMean-field theory
๐กPhase diagram
๐กQuantum spin liquid
Highlights
Dr. Lin from UC Berkeley discusses the story on Kagome lattice and the discovery of a phase with interesting electronic properties.
The talk is based on their research published in Physical Review and available for interested attendees.
Dr. Lin acknowledges the Birley group and his advisor Jore for their contributions to the work.
The presentation outlines the background, introduction to frustrated systems, focusing on the Kagome flatband.
The study explores repulsive electrons on the flatband and their effects using a pure Hubbard model.
The introduction of extended repulsion in the model reveals new phases and faces.
Dr. Lin presents theoretical work with practical relevance, suggesting possible experimental observations.
The talk delves into the background of interacting electrons in crystal structures and the effects of interaction U.
The concept of symmetry breaking and its characterization by an order parameter Delta is explained.
Examples of symmetry breaking orders such as ferromagnetism and spin density waves are discussed.
The search for strong interacting electron phases and the significance of the flatband in this context are highlighted.
Dr. Lin explains how to estimate the strength of interacting electron phases using the interacting window.
The interest in flatbands over the past decade and their potential for hosting strongly interacting electron phases are covered.
The presentation identifies frustrated systems as promising candidates for realizing flatbands.
The reasons behind the flatbands in certain materials, such as destructive interference, are explored.
The identification of flatbands in kagome compounds and their relevance to experiments are discussed.
The potential for observing ferromagnetism and charge density wave in iron germanium is suggested.
Dr. Lin proposes that reducing correlation in materials could lead to the observation of non-collinear spin orders.
The possibility of observing Z2 spin liquids beyond mean-field theory is mentioned.
The talk concludes with a summary of the mean-field analysis on the kagome flatband and its findings.
Transcripts
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